Calculations of Crystallization Temperature of Multicomponent Metallic Glasses

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A model for calculating crystallization temperature (<I>T</I><SUB>x</SUB>) of multicomponent metallic glasses is proposed by modifying the Miedema’s model which is used for calculating <I>T</I><SUB>x</SUB> of binary systems. The calculations were carried out for nearly 900 metallic glasses including 470 binary and 398 ternary alloys. In the present model, the cavity formation energy (<I>ΔH</I><SUB>cavity</SUB><SUP>for</SUP>) for multicomponent metallic glasses was theoretically derived on the basis of the Miedema’s model. The equation for expressing the relation between experimental <I>T</I><SUB>x</SUB> and theoretical <I>ΔH</I><SUB>cavity</SUB><SUP>for</SUP> was statistically analyzed by the least-squares method, yielding <I>T</I><SUB>x</SUB>=4.16×<I>ΔH</I><SUB>cavity</SUB><SUP>for</SUP>+318. The binary and ternary systems tend to show different equations between <I>T</I><SUB>x</SUB> and <I>ΔH</I><SUB>cavity</SUB><SUP>for</SUP>. The inherent equation in each system was analyzed as simultaneous achievement of the increase in stability of metallic glasses and decrease in <I>ΔH</I><SUB>cavity</SUB><SUP>for</SUP> due to multicomponent alloying. Furthermore, the glass-forming ability was predicted by reduced crystallization temperature instead of reduced glass transition temperature. As a result, it was found that reduced crystallization temperature can be calculated close to reduced glass transition temperature except for Pt-, Pd- and La-based systems. It is of great importance that <I>T</I><SUB>x</SUB> can be calculated for multicomponent metallic glasses by semi-empirical method.

収録刊行物

  • Materials transactions

    Materials transactions 43(9), 2275-2284, 2002-09-01

    公益社団法人 日本金属学会

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  • Calculations of Mixing Enthalpy and Mismatch Entropy for Ternary Amorphous Alloys

    Takeuchi Akira , Inoue Akihisa

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