VARIATIONS OF CARBON ISOTOPIC RATIO OF ATMOSPHERIC CARBON DIOXIDE OVER JAPAN

  • NAKAZAWA Takakiyo
    Center for Atmospheric and Oceanic Studies, Faculty of Science, Tohoku University
  • MORIMOTO Shinji
    Center for Atmospheric and Oceanic Studies, Faculty of Science, Tohoku University
  • AOKI Shuhji
    National Institute of Polar Research
  • TANAKA Masayuki
    Center for Atmospheric and Oceanic Studies, Faculty of Science, Tohoku University

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抄録

Carbon dioxide samples collected in the troposphere over Japan during the periods from April 1984 to November 1990 were analyzed for the carbon isotope ratio, δ^<13>C, with a precision of 0.03‰ (one standard deviation). The seasonal cycle of δ^<13>C decreased with increasing height, with a phase delay of about one month between the lower and upper troposphere, which was quite similar to that of the CO_2 concentration. It was found from the observed seasonal cycles of the CO_2 concentration and δ^<13>C that the rate of change in δ^<13>C with respect to the CO_2 concentration is about -0.05‰ per ppmv. This implies that the seasonal CO_2 cycle over Japan is mainly induced by seasonally dependent biospheric activities. However, the air transport from different latitudes is also important for the seasonal CO_2 cycle, especially in the upper troposphere. δ^<13>C decreased secularly at an average rate of about -0.03‰ per year due mainly to combustion of fossil fuels with lighter CO_2 relative to the atmospheric CO_2. Irregular variations of δ^<13>C with the periods of two or three years, superimposed on the secular trend, were also observed; they were almost in phase with these of the CO_2 concentration. From the comparison of both irregular variations, it was found that the cause could primarily attributed to the imbalance in CO_2 exchange between the atmosphere and biosphere in association with climate change, rather than between the atmosphere and oceans.

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詳細情報 詳細情報について

  • CRID
    1571698601806252544
  • NII論文ID
    110001025948
  • NII書誌ID
    AA10756213
  • ISSN
    09142037
  • 本文言語コード
    en
  • データソース種別
    • CiNii Articles

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