Spatial Optical Parametric Coupling of Picosecond Light Pulses and Transverse Relaxation Effect in Resonant Media

  • Yajima Tatsuo
    The Institute for Solid State Physics, The University of Tokyo
  • Taira Yoichi
    The Institute for Solid State Physics, The University of Tokyo

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  • Spatial Optical Parametric Coupling of

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The dynamical properties of a third-order nonlinear optical process, in which two incident light pulses with wave vectors k1 and k2 generate a light wave with 2k2k1 in resonant media, are discussed with particular attention to the effect of transverse relaxation time T2. It is shown that the correlation trace (output light energy vs incident pulse separation) for this process provides a general means of obtaining information on ultrashort T2 for both the homogeneously and inhomogeneously broadened transitions, and for both tp(pulse width)<T2 and tp>T2. An experimental demonstration for tp>T2 is given by using a dye molecule and a picosecond light source.

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