Development of Time-Resolved Scanning Tunneling Microscopy in Femtosecond Range.

  • Takeuchi Osamu
    Institute of Applied Physics, CREST, University of Tsukuba, Tsukuba 305-8573, Japan
  • Morita Ryuji
    Department of Applied Physics, CREST, Hokkaido University, Sapporo 060-8628, Japan
  • Yamashita Mikio
    Department of Applied Physics, CREST, Hokkaido University, Sapporo 060-8628, Japan
  • Shigekawa Hidemi
    Institute of Applied Physics, CREST, University of Tsukuba, Tsukuba 305-8573, Japan

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A promising design for achieving the ultimate spatial and temporal resolution is proposed. With modulation of the time delay between two femtosecond laser pulses repeatedly illuminating a scanning tunneling microscope junction, the induced component of the tunneling current is detected as a function of the delay time. With this method, a high signal-to-noise ratio, stable measurement free from fluctuation of laser intensity, and removal of the thermal expansion effect can be achieved. Using the photovoltage effect of GaAs, the high performance of the newly developed system is demonstrated in the femtosecond range.

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