Electronic Properties of Graphite-Potassium intercalation Compounds. II. Resistivity, Hall Effect and Magnetoresistance

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Resistivity (ρ), Hall coefficient (RH) and transverse magnetoresistance (tMR) of C8K(1st) and C12NK(N-th stage, N=2, 3 and 4) at temperatures of 1.2 to 300 K have been investigated in connection with the study of the Fermi surfaces (Part I). Resistivities in the N≥2 stage compounds show some anomalies which are associated with the order-disorder phase transitions. In C8K, ρ has a temperature dependence of a+bT+cT2. The temperature dependence of RH indicates the one-electron conduction for the N≥2 compounds and the two-carriers one for C8K. The tMR of each compound is represented by a linear function of magnetic field at about 4 to 15 T. The angular dependence of tMR indicates the cylindrical Fermi surface in a whole. The charge transfer rate from potassium to the graphite band is evaluated as 0.1 to 0.4 electron per atom for the 1st to 4th stage compounds.

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