Raman Scattering and Dilatometric Studies of a Molecular Crystal Chloranil(C6Cl4O2)

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  • Wada Mitsuo
    Synthetic Crystal Research Laboratory, Faculty of Engineering, Nagoya University
  • Shichi Hiroyasu
    Synthetic Crystal Research Laboratory, Faculty of Engineering, Nagoya University
  • Sawada Akikatsu
    Synthetic Crystal Research Laboratory, Faculty of Engineering, Nagoya University
  • Ishibashi Yoshihiro
    Synthetic Crystal Research Laboratory, Faculty of Engineering, Nagoya University

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  • Raman Scattering and Dilatometric Studies of a Molecular Crystal Chloranil (C<SUB>6</SUB>Cl<SUB>4</SUB>O<SUB>2</SUB>)
  • Raman Scattering and Dilatometric Studi

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The Raman scattering spectra and the thermal expansions of chloranil crystal were measured below and above the phase transition point T0=93.8 K. The index of the transition parameter was obtained from the temperature dependence of the soft mode frequency for 0.08<(T0−T)⁄T0<0.89 as β=0.47±0.05, including within its range the mean-field value 0.5.

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