Phase Diagram of a Quasi-One-Dimensional Antiferromagnet (CH<SUB>3</SUB>)<SUB>4</SUB>NMnCl<SUB>3</SUB>(TMMC)

  • Takeda Kazuyoshi
    Department of Material Physics, Faculty of Engineering Science, Osaka University
  • Koike Tomoyuki
    Department of Material Physics, Faculty of Engineering Science, Osaka University
  • Tonegawa Takashi
    Department of Physics, Faculty of Science, Kobe University

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The magnetic phase diagram of the most typical quasi-one-dimensional antiferromagnet (CH3)4NMnCl3(TN=0.835 K) has been established. An anisotropic axis has been found in the hexagonal plane perpendicular to c-axis. When the magnetic field H is applied along the easy axis in the plane, the Néel temperature TN(H) shifts down to the bicritical point at (Tb=0.5 K, Hb=11.4 kG) on the (T-H) diagram, and for H>Hb, TN(H) turns to increase monotonously. TN(H) for the hard axis shows an anomalous increase as has been reported experimentally and theoretically for quasi-one-dimensional antiferromagnets.

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