Adsorption of ^<188>Re Complexes with Aminomethylenephosphonate on Hydroxyapatite

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The adsorption properties of newly developed <SUP>188</SUP>Re complexes with aminomethylenephosphonate (amp) (EDTMP-Ethylenediamine-N, N, N', N'-tetrakis(methylenephosphonic acid), EDBMP-Ethylenediamine-N, N'-bis(methylenephosphonic acid) and NTMP-Nitrilotris(methylenephosphonic acid)) on hydroxyapatite was investigated. The adsorption of <SUP>188</SUP>Re complexes was strongly affected by pH and ionic strength in a solution. The adsorption coefficient(ml/g), which is defined by the ratio of the concentration of the complex per unit weight of the hydroxy-apatite to the concentration in unit volume of the solution, increased with decreasing pH and ionic strength. These observations suggest that one of the causes of the adsorption of <SUP>188</SUP>Re-amp is considered to be the electrostatic forces between the negative <SUP>188</SUP>Re-amp complex and the positive HAP surface. The adsorption affinity of the <SUP>188</SUP>Re-amp complex for HAP increased in the order of <SUP>188</SUP>Re-EDBMP<<SUP>188</SUP>Re-NTMP<<SUP>188</SUP>Re-EDTMP. Furthermore, the adsorption coefficient of carrier-free <SUP>188</SUP>Re-EDTMP was larger than that of carrier-added one under the same conditions. From a detailed comparison of the effect of the Re carrier concentration on the adsorption coefficient of <SUP>188</SUP>Re-EDTMP with its structural analysis by HPLC, we concluded that the Re carrier effect on the adsorption coefficient was caused by the different distribution of the components in the <SUP>188</SUP>Re-EDTMP mixture between the carrier-free and the carrier-added complex.

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  • Journal of Nuclear and Radiochemical Sciences

    Journal of Nuclear and Radiochemical Sciences 2(1), 5-9, 2001-12-01

    日本放射化学会

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各種コード

  • NII論文ID(NAID)
    10013977586
  • NII書誌ID(NCID)
    AA11948402
  • 本文言語コード
    ENG
  • 資料種別
    ART
  • ISSN
    13454749
  • データ提供元
    CJP書誌  J-STAGE 
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