レーザーと放射光による2光子励起分光法

書誌事項

タイトル別名
  • Two-Photon Spectroscopy Using Laser Light and Synchrotron Radiation
  • レーザー ト ホウシャコウ ニ ヨル 2 コウシレイキブンコウホウ

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The accessibility of the two-photon spectroscopy to the forbidden states of the one-photon transition makes ita powerful tool. The two-photon excited core excitons were chosen as an example of a combinational use oflaser light and synchrotron radiation. The experiments were performed at Beamline 1B of UVSOR, Institutefor Molecular Science. The two light sources were synchronized at a repetition rate of 90 MHz. The singlephotoncounting method was used for detecting luminescence as the signal of two-photon absorption by thesample. The two-photon excitation spectrum of Auger-free luminescence from the BaF2 crystal exhibits severalpeaks due to core excitons. The analysis of the spectrum reveals the spin-orbit splitting and dispersion ofthe 4f and 6p states of the Ba ion in BaF2. The lifetime of the core exciton is obtained from the time-resolvedmeasurements.

収録刊行物

  • レーザー研究

    レーザー研究 34 (8), 549-554, 2006

    一般社団法人 レーザー学会

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