Effects of Convective and Diffusive Mixing on a Periodic Reaction

  • Daimon Sakiko
    Division of Chemical Engineering, Graduate School of Engineering Science, Osaka University
  • Okada Buntaro
    Division of Chemical Engineering, Graduate School of Engineering Science, Osaka University
  • Hirata Yushi
    Division of Chemical Engineering, Graduate School of Engineering Science, Osaka University
  • Inoue Yoshiro
    Division of Chemical Engineering, Graduate School of Engineering Science, Osaka University

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Other Title
  • 周期反応系に及ぼす対流・拡散混合の影響
  • シュウキ ハンノウケイ ニ オヨボス タイリュウ カクサン コンゴウ ノ エイキョウ

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Abstract

To clarify the influence of mixing on chemical reactions, the effects of convective and diffusive mixing on the spatiotemporal structure of the concentration field in a Lotka-Volterra periodic reaction is analyzed. At the beginning of mixing, concentration distribution is not uniform spatially, and the oscillation mode differs at every position. After a long time, however, the concentration becomes uniform throughout a whole system, and then synchronizes and oscillates with a unique period. The whole concentration field is regarded as an assembly of concentration oscillators. This assembly is a dynamical network of short-range interactions due to diffusion and recombination caused by convective flow. With this model, the process to final coherent oscillation mode and the factors affecting on it were analyzed.

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