Palladium-catalyzed Regio- and Diastereoselective Allylic Alkylation in Ionic Liquids

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  • Motoi Kawatsura
    Department of Chemistry and Biotechnology, Graduate School of Engineering, Tottori University
  • Hideyuki Nobuto
    Department of Chemistry and Biotechnology, Graduate School of Engineering, Tottori University
  • Shunsuke Hayashi
    Department of Chemistry and Biotechnology, Graduate School of Engineering, Tottori University
  • Takuya Hirakawa
    Department of Chemistry and Biotechnology, Graduate School of Engineering, Tottori University
  • Daiji Ikeda
    Department of Chemistry and Biotechnology, Graduate School of Engineering, Tottori University
  • Toshiyuki Itoh
    Department of Chemistry and Biotechnology, Graduate School of Engineering, Tottori University

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<jats:title>Abstract</jats:title> <jats:p>Palladium-catalyzed regio- and diastereoselective allylic alkylations using ionic liquids (ILs) as a solvent were demonstrated. The reaction using diethyl(2-methoxyethyl)methylammonium bis(trifluoromethanesulfonyl)amide ([N221ME][NTf2]) or ethylhexyldimethylammonium bis(trifluoromethanesulfonyl)amide ([N6211][NTf2]) as solvent realized the recyclable use of the palladium catalyst while maintaining excellent regioselectivity and diastereoselectivity.</jats:p>

収録刊行物

  • Chemistry Letters

    Chemistry Letters 40 (9), 953-955, 2011-09

    Oxford University Press (OUP)

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