New Stacking Variations of the Charge and Orbital Ordering in the Metal-Ordered Manganite YBaMn<sub>2</sub>O<sub>6</sub>

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  • Kageyama H.
    Material Design and Characterization Laboratory, Institute for Solid State Physics, University of Tokyo
  • Nakajima T.
    Material Design and Characterization Laboratory, Institute for Solid State Physics, University of Tokyo
  • Ichihara M.
    Material Design and Characterization Laboratory, Institute for Solid State Physics, University of Tokyo
  • Ueda Y.
    Material Design and Characterization Laboratory, Institute for Solid State Physics, University of Tokyo
  • Yoshizawa H.
    Neutron Scattering Laboratory, Institute for Solid State Physics, The University of Tokyo
  • Ohoyama K.
    Institute for Materials Research, Tohoku University

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  • New Stacking Variations of the Charge and Orbital Ordering in the Metal-Ordered Manganite YBaMn2O6.

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We performed transmission electron microscopy (TEM) and powder neutron diffraction experiments on an A-site ordered manganese perovskite YBaMn2O6 which undergoes unusual and multiple phase transitions. In the paramagnetic insulating phase, the so-called CE type of charge and orbital ordering was observed in the monoclinic a–b plane, which has been frequently observed for the ordinary solid solution of A1−x3+Ax′2+MnO3 around x=0.5. TEM revealed, however, a fourfold periodicity along the c axis, suggesting a new stacking pattern, in which planes of the CE type are built up according to the sequence [ααββ…]. Interestingly, when the system entered the antiferromagnetic state below 195 K, this stacking pattern changed into [αααα…] or [αβαβ…], suggesting a close interplay between spins and orbitals. The obtained stacking patterns were strongly correlated to the inherent structural alternation, i.e., the Y/Ba order along the c axis.

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