Z2 Vortex-Induced Broadening of the EPR Linewidth in the Two-Dimensional Triangular Lattice Antiferromagnets,HCrO2 and LiCrO2

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  • Z<SUB>2</SUB> Vortex-Induced Broadening of the EPR Linewidth in the Two-Dimensional Triangular Lattice Antiferromagnets, HCrO<SUB>2</SUB> and LiCrO<SUB>2</SUB>
  • Z2 Vortex Induced Broadening of the EPR

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The title compounds are the family of the AMO2-type (R\bar3m) crystal which has a pronounced layer structure and are promising candidates for the two-dimensional Heisenberg triangular lattice antiferromagnet (2DH TAL–AF). The interesting observation is that a singular point of the EPR signal is located around TKM=0.66JS2 for the critical temperature of phase transition associated with the pairing-dissociation of the Z2 vortices, suggesting the present system behaves as 2DH TAL–AF down to very close to TKM. The EPR linewidth exhibits Z2 vortex-induced broadening above the critical temperature which is inversely proportional to the thermally excited vortex density, nv∝exp (−EvkBT) with the activation energy Ev≅4kBTKM.

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