Pressure-induced Magnetic Quantum Phase Transition from Gapped Ground State in TlCuCl3

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  • Pressure-induced Magnetic Quantum Phase Transition from Gapped Ground State in TlCuCl<sub>3</sub>

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Abstract

Magnetization measurements under hydrostatic pressure were performed on an S=1⁄2 coupled spin dimer system TlCuCl3 with a gapped ground state under magnetic field H parallel to the [201] direction. With increasing applied pressure P, the gap decreases and closes completely at Pc=0.42±0.05 kbar. For P>Pc, TlCuCl3 undergoes antiferromagnetic ordering. A spin-flop transition was observed at Hsf\\simeq0.7 T. The spin-flop field is approximately independent of pressure, although the sublattice magnetization increases with pressure. The gap and Néel temperature are presented as functions of pressure. The occurrence of the pressure-induced quantum phase transition is attributed to the relative enhancement of the interdimer exchange interactions compared with the intradimer exchange interaction.

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