Possible Coexistence of Quadrupolar and Magnetic Ordering in Ce<sub>0.7</sub>Pr<sub>0.3</sub>B<sub>6</sub>

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  • Possible Coexistence of Quadrupolar and Magnetic Ordering in Ce0.7Pr0.3B6

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We have investigated the physical properties of Ce0.7Pr0.3B6 in order to clarify the doping effect on the multipolar interactions in CeB6 and PrB6. As a result of the suppression of the antiferro-quadrupolar ordering temperature TQ and the enhancement of TN by Pr doping, six long-range ordered (LRO) phases appear. TQ exhibits a smooth increase with increasing magnetic field as in CeB6. At a high magnetic field, above ∼10 T, only phase II exists. As for the three LRO phases below ∼10 T and below TQ, there exists a possibility of incommensurate quadrupolar and magnetic ordering. A new question of how the quadrupolar ordering is compatible with the magnetic ordering appears in the present study. The coexistence of the magnetic and quadrupolar orderings in Ce0.7Pr0.3B6 indicates that the strong Ce–Pr interaction is different from the weak Ce–Nd interaction in CexNd1−xB6.

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