Ultrafast Photoinduced Formation of Metallic State in a Perovskite-type Manganite with Short Range Charge and Orbital Order

  • Okimoto Yoichi
    Correlated Electron Research Center (CERC), National Institute of Advanced Industrial Science and Technology (AIST)
  • Matsuzaki Hiroyuki
    Department of Advanced Materials Science, University of Tokyo
  • Tomioka Yasuhide
    Correlated Electron Research Center (CERC), National Institute of Advanced Industrial Science and Technology (AIST)
  • Kezsmarki Istvan
    Department of Applied Physics, University of Tokyo
  • Ogasawara Takeshi
    Correlated Electron Research Center (CERC), National Institute of Advanced Industrial Science and Technology (AIST)
  • Matsubara Masakazu
    Correlated Electron Research Center (CERC), National Institute of Advanced Industrial Science and Technology (AIST)
  • Okamoto Hiroshi
    Correlated Electron Research Center (CERC), National Institute of Advanced Industrial Science and Technology (AIST) Department of Advanced Materials Science, University of Tokyo
  • Tokura Yoshinori
    Correlated Electron Research Center (CERC), National Institute of Advanced Industrial Science and Technology (AIST) Department of Applied Physics, University of Tokyo

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Abstract

Femtosecond reflection spectroscopy was performed on a perovskite-type manganite, Gd0.55Sr0.45MnO3, with the short-range charge and orbital order (CO/OO). Immediately after the photoirradiation, a large increase of the reflectivity was detected in the mid-infrared region. The optical conductivity spectrum under photoirradiation obtained from the Kramers–Kronig analyses of the reflectivity changes demonstrates a formation of a metallic state. This suggests that ferromagnetic spin arrangements occur within the time resolution (∼200 fs) through the double exchange interaction, resulting in an ultrafast CO/OO to FM switching.

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