The Effect of Randomness on the Quantum Spin System Tl<SUB>1−<I>x</I></SUB>K<I><SUB>x</SUB></I>CuCl<SUB>3</SUB> with <I>x</I>=0.44 Studied by the Zero-Field Muon-Spin-Relaxation (ZF-μSR) Method

  • Suzuki Takao
    Advanced Meson Science Laboratory, RIKEN (The Institute of Physical and Chemical Research)
  • Yamada Fumiko
    Department of Physics, Tokyo Institute of Technology
  • Watanabe Isao
    Advanced Meson Science Laboratory, RIKEN (The Institute of Physical and Chemical Research)
  • Goto Takayuki
    Department of Physics, Sophia University
  • Oosawa Akira
    Department of Physics, Sophia University
  • Tanaka Hidekazu
    Department of Physics, Tokyo Institute of Technology

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  • The effect of randomness on the quantum spin system Tl1-xKxCuCl3 with x = 0.44 studied by the zero-field muon-spin-relaxation (ZF-μSR) method
  • The effect of randomness on the quantum spin system Tl1 xKxCuCl3 with x 0 44 studied by the zero field muon spin relaxation ZF mSR method
  • The Effect of Randomness on the Quantum Spin System Tl<sub>1-<i>x</i></sub>K<sub><i>x</i></sub>CuCl<sub>3</sub> with <i>x</i>=0.44 Studied by the Zero-Field Muon-Spin-Relaxation (ZF-µSR) Method

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Abstract

Zero-field muon-spin-relaxation (ZF-μSR) measurements were carried out down to 80 mK on the randomness bond system Tl1−xKxCuCl3 with x=0.44. Time spectra are well fitted by the stretched exponential function exp(−λt)β. The muon spin relaxation rate λ increases rapidly with decreasing temperature, and β tends to 0.5 at 80 mK. The divergent increase of λ suggests the critical slowing down of the frequency of the Cu-3d spin fluctuations toward a spin frozen state below 80 mK, and the root-exponential-like behavior of the time spectrum indicates that the origin of the relaxation is possibly the spatially-fixed fluctuating dilute moments.

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