Exciton dephasing and multiexciton recombinations in a single carbon nanotube

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We studied the temperature and excitation intensity dependence of exciton luminescence in individual single-walled carbon nanotubes (SWNTs) using single nanotube photoluminescence (PL) spectroscopy. The linear temperature dependence of the PL linewidth in a single SWNT implies that the exciton dephasing is dominated by the interaction between the exciton and the phonon mode with very low energy under lower-excitation conditions. Saturation of the PL intensity and broadening of the PL linewidth in a single SWNT occur simultaneously with an increase in excitation laser intensity. Our findings show that the rapid exciton-exciton annihilation through multiparticle Auger recombination broadens the homogeneous PL linewidth.

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詳細情報 詳細情報について

  • CRID
    1050001202063198464
  • NII論文ID
    120001682385
  • ISSN
    10980121
  • HANDLE
    2433/87354
  • 本文言語コード
    en
  • 資料種別
    journal article
  • データソース種別
    • IRDB
    • CiNii Articles

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