Unified explanation for linear and nonlinear optical responses in β-carotene : A sub-20−fs degenerate four-wave mixing spectroscopic study

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The four-wave mixing signal of β-carotene measured under the resonant excitation is reported. A clear coherent oscillation with a period of a few tens of femtoseconds was observed. We have estimated the line broadening function required to simulate this oscillation behavior. The parameters, including the solvation effect, which are essential for calculating the optical signals have also been determined. The validity of our simulation has been evaluated by comparing the theoretically calculated linear and nonlinear optical signals with the experimental results....

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  • Physical Review B

    Physical Review B 75 (15), 155110-, 2007-04-20

    American Physical Society

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