High-temperature dielectric responses of molecularly-thin titania nanosheet

DOI Web Site 被引用文献3件 参考文献24件
  • KIM Yoon-Hyun
    International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS) Graduate School of Advanced Science and Engineering, Waseda University
  • OSADA Minoru
    International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS) Graduate School of Advanced Science and Engineering, Waseda University
  • DONG Lei
    International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS) Graduate School of Advanced Science and Engineering, Waseda University
  • KIM Hyung-Jun
    International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS)
  • SASAKI Takayoshi
    International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS)

抄録

We have investigated high-temperature dielectric properties of titania nanosheet (Ti0.87O2), a new class of high-κ nanomaterials derived from the exfoliation of layered compounds. In-situ characterizations using atomic force microscopy indicate a robust insulating property in a monolayer form of Ti0.87O2 nanosheets even at 200°C. Furthermore, layer-by-layer assembled nanocapacitors exhibit both size-free high-εr characteristic (~120) and high insulation resistance (~10−7 A/cm2) at high temperatures up to 250°C. The simultaneous improvement of εr and thermal stability in high-κ nanodielectrics is of critical importance for applications of high-temperature capacitors.

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