Effect of La Impurities on the Phase Transitions in PrFe<SUB>4</SUB>P<SUB>12</SUB>

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  • Effect of La impurities on the phase transitions in PrFe4P12

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Abstract

The effect of La impurities on the low-field (A phase) and high-field (B phase) ordered states in PrFe4P12 has been studied using dc magnetization measurements on a series of Pr1−xLaxFe4P12 (x=0, 0.01, 0.05, and 0.15). It is found that the long-range A phase order evolves to a short-range one at a very small La concentration between x=0.01 and 0.05. We also find clear evidence for the existence of ferromagnetism in the sample with x≥0.05. Remarkably, the ferromagnetic ordering temperature TC increases from 1.05 K for x=0.05 to 1.45 K for x=0.15, although the Weiss temperature decreases with increasing x. These observations indicate the competition between the A phase and ferromagnetic state, and the role of nesting on the A phase transition is emphasized.

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