Kinetic Studies on the Reactions of Atomic Oxygen with Furan, 2-Methylfuran, and 2,5-Dimethylfuran at Elevated Temperatures

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  • Haruka Yoshizawa
    Department of Materials and Life Sciences, Sophia University, 7-1 Kioi-cho, Chiyoda-ku, Tokyo 102-8554
  • Hiroki Nagashima
    Department of Materials and Life Sciences, Sophia University, 7-1 Kioi-cho, Chiyoda-ku, Tokyo 102-8554
  • Yoshinori Murakami
    Department of Materials Engineering, Nagaoka College, National Institute of Technology, 888 Nishikatakai, Nagaoka, Niigata 940-8532
  • Kazuo Takahashi
    Department of Materials and Life Sciences, Sophia University, 7-1 Kioi-cho, Chiyoda-ku, Tokyo 102-8554

抄録

<jats:title>Abstract</jats:title> <jats:p>The reactions of O(3P) atoms with furan, 2-methylfuran (2-MF), and 2,5-dimethylfuran (2,5-DMF) were studied at elevated temperatures by using a shock tube technique coupled with atomic resonance absorption spectroscopy (ARAS). The rate coefficients (k) determined from the time profiles of O(3P) atoms were expressed by the relation of kO+2,5-DMF &gt; kO+2-MF &gt; kO+FURAN. The molecular orbital calculations with CBS-QB3 level were also performed and the possible product channels of these reactions were discussed.</jats:p>

収録刊行物

  • Chemistry Letters

    Chemistry Letters 46 (8), 1207-1210, 2017-05-30

    Oxford University Press (OUP)

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