Vibrations at surfaces : proceedings of the third international conference, Asilomar, California, U.S.A., 1-4 September, 1982

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Vibrations at surfaces : proceedings of the third international conference, Asilomar, California, U.S.A., 1-4 September, 1982

editors, C.R. Brundle and H. Morawitz

（Studies in surface science and catalysis, 14）

Elsevier Scientific Pub. Co. , Distributors for the U.S. and Canada, Elsevier Science Pub. Co., 1983

Uniform Title

Journal of electron spectroscopy and related phenomena

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Papers presented at the third International Conference on "Vibrations at Surfaces" (VAS III), held at Asilomar, Calif., from Sept. 1-4, 1982

"Reprinted from the Journal of electron spectroscopy and related phenomena, v. 29 (Part A) and 30 (Part B)."

Includes bibliographical references and indexes

Description and Table of Contents

Description

Studies in Surface Science and Catalysis 14: Vibrations at Surfaces documents the proceedings of the third International Conference on ""Vibrations at Surfaces"" held at Asilomar, California, from September 1-4, 1982. Almost all of the 102 papers presented at the meeting are published in this volume. The topics chosen for the eight sessions held over a span of three days were: (I) Vibrational Frequency Shifts and Widths-Lateral Interactions; (II) Dynamical Processes at Surfaces; (III) and (IV) Electron Loss Spectroscopy; (V) Raman and Surface Enhanced Raman Scattering; (VI) Infrared Absorption and Reflection Spectroscopy; (VII) Beam Surface Scattering Surface Phonons; (VIII) Electron Tunneling Spectroscopy - Surface Enhanced Raman Studies in Electrochemistry. In addition, C. B. Duke presented an introductory keynote surveying progress in the field since the last meeting. In the final session H. Ibach and T. Grimley presented conference overviews and future prospects for the field from an experimental and theoretical perspective. Also included in the Proceedings are four literature surveys on Energy Loss, Inelastic Tunneling, Infrared and Raman (SERS) papers.

Table of Contents

  • Part AForewordList of ParticipantsIntroductory Keynote Hot Atoms and Cold Facts: Mysteries and Opportunities in Vibration-Assisted Surface ChemistrySession I: Vibrational Frequency Shifts and Widths
  • Lateral Interactions Phase and Bonding Transitions in Chemisorbed Layers Studied by Vibrational Frequency Shifts Combined Vibrational/Temperature Programmed Reaction Spectroscopy Studies of Reaction Intermediates on Metal Surfaces High Resolution Infrared Study of Hydrogen Chemisorbed on Si(100) Thermal Scattering of Slow Electrons During Elastic Specular Reflection from a Cu(001) Surface Lateral Interactions and Vibrational Lifetimes The Oxidation of Methanol on Cu(100) Studied by Infrared Spectroscopy Vibrations Spectra of Oxygen Chemisorbed on Nickel(110) Surfaces Dipole-Dipole Coupling in Adsorbate Vibrational Mode Spectra The Reflection-Absorption Infrared Spectrum of the Dioxygen Species Adsorbed on Platinum recorded by FT-IR Spectroscopy Ab Initio CI Investigation of Hydrogen Atom Adsorption on Li Clusters: Embedded Cluster Model Investigation of Lateral Interactions in ChemisorptionSession II: Dynamical Processes at Surfaces Energy Dissipation at Metal Surfaces: Electronic Versus Vibrational Excitations Selective Desorption from the Binary Coadsorbate C2,H6-CH3F-NaCI by Resonant Vibrational Excitation with Laser Infrared Radiation Laser-Induced Thermal Desorption of CO from Clean Polycrystalline Copper: Time-of-Flight and Surface Diffusion Measurements Infrared Emission Spectroscopy of Co on Ni Electronic Damping of the Motion of Adsorbates on Metal Surfaces Infrared Laser Stimulated Surface Processes The Exposure Dependence and Emission Spectrum of Chemiluminescence Produced During the Oxidation of Si(111) by O2 Laser-Induced Decomposition of Sodium Azide Non-Equilibrium Behavior on Pulsed Laser Evaporated Surfaces Surface Vibration Correlation with d-Electron (Hole) Per Atom Ratio (d-Bandfilling) in CO Chemisorption on Supported Transition Metal Particles: Dominance of Hund's Rule and d-Electron Degeneracy in Real Supported Catalysts Vibrational State of Chemisorbed Molecule on Metal SurfaceSession III: Electron Energy Loss Spectroscopy High Resolution Electron Energy Loss Studies of Adsorbates Utilizing Impact and Resonance Scattering High Resolution EELS Studies of Clean and Oxide Covered Semiconductor Surfaces The Chemisorption of Nitrogen on the (001) Surface of Ruthenium Adsorbate Structure Modeling Based on EELS and Lattice Dynamical Calculations: Application to 0/A1(111) Summary Abstract: Vibrational Excitations of Hydrogen and Oxygen on Pd(100) High Resolution Electron Energy Loss Spectroscopic Study of the Interaction of Oxygen with Magnesium Single Crystal Surfaces Low Frequency Surface Resonance Modes in Electron Loss Spectroscopy Oxygen Adsorption on the Kinked Pt(321) Surface Calculation of the EELS Spectra of the Ni(001) surface with p(2X 2) and c(2X 2) Overlayers of Oxygen Theoretical Calculation of Vibrations of Adsorbed Species Contrasting Bonding Configurations of Acetone on Pt(111) and Ru(001) Surfaces The Methoxy Intermediate on Mo(100): Effects of Surface Oxidation HREELS Studies of Adsorbates on Polar Solids: Water on SrTiO3(100) A Vibrational Study of Ammonia Chemisorbed on Ni(110) and Ni(111): Whither Goest the Metal-Nitrogen Stretching Mode on FCC(111) Surfaces? The Adsorption of NO on Ru(001) and Its Co-Adsorption with Oxygen Studied by Vibrational SpectroscopySession IV: Electron Energy Loss Spectroscopy II The Adsorption of Ammonia on a Fe(110) Single Crystal Surface Studied by High Resolution Electron Energy Loss Spectroscopy (EELS) Spatial Intensity Distributions from Electron Impact Scattering Modes: W(100)(1x1)H Hydrogen Chemisorption of Ni(110) by High-Resolution Electron Energy Loss Spectroscopy Identification of Surface Vibrations on Clean and Oxygen Covered Pt(111) Surfaces with High Resolution Electron Energy Loss Spectroscopy (EELS) Vibrational Spectroscopy Using HREELS of Benzene Adsorbed on the Rh(111) Crystal Surface HREELS Study of Formic Acid Adsorption on Gold (110) and (111) Surfaces The Adsorption and Dehydrogenation of Cyclopentane on Ru(001) Thermal Evolution of C2H2 and C4H2 on Pd(111) Studied by High-Resolution Electron Energy Loss Spectroscopy Electronic Transitions of Ar, Xe, N2, CO Physisorbed on Ag(111) and AI(111) Vibrational Spectra of Ethylene and Acetylene on Metal Surfaces - an Electron Energy Loss Study of Ethylene Adsorbed on Ni(110) and Its Carbided Surface, and the Use of Metal-Cluster Analogies Electron Energy Loss Spectroscopy of the Decomposition of Formic Acid on Ru(001) Azimuthal Dependence of Impact Scattering in Electron Energy Loss SpectroscopySession V: Raman and Surface Enhanced Raman Scattering On the Contribution of Charge Transfer Excitations to SERS Multichannel Raman Spectroscopy of Unroughened Noble Metal and Non-Noble Metal Films and Tunnel Junctions Charge Transfer Effects in Surface Enhanced Raman Scattering Orientation Dependence of Surface Enhanced Raman Intensities: Results from Ab Initio Calculations Surface Enhanced Raman Scattering (SERS) from Silver, Copper and Gold Films in UHV: Excitation Spectra A Comparison of Raman Scattering, Resonance Raman Scattering and Fluorescence from Molecules Adsorbed on Silver Island Films Using Surface Enhanced Raman Scattering to Study Vibrations of Adsorbates on Thin Metallic Overlayers on Silver Influence of Foreign Metal Atoms Deposited at Electrodes on Local and Non-Local Processes in Surface Enhanced Raman Scattering Surface Raman Spectroscopy without Enhancement: Pyridine on Ag(111) Raman Spectra of Pyridine Adsorbed on Ni(111) Surface Enhanced Raman Spectroscopy of Palladium Acetylene Adsorption on Silver Films: A Raman Vibrational Study The SERS Phenomenon in Light of Recent Excitation Profile Measurements Exact Calculations of Scattering and Enhanced Fields of Electromagnetic Waves on Grating SurfacesPart BSession VI: Infrared Absorption and Reflection Spectroscopy Infrared Spectroscopy of Adsorbates on Low-Area Surfaces: The Advantage of a Photons-in, Photons-out Technique The Application of Reflection Infrared and Surface Enhanced Raman Infrared Specular Reflection and SERS Spectra of Molecules Adsorbed on Smooth Surfaces Surface Photoacoustic Spectroscopy - a New Technique for the Study of Surface Vibrations Enhanced Adsorbate Raman Scattering and Surface Plasmon Radiation Theoretical Vibrational Frequencies for NHx and CHx Reactive Intermediates on Nickel(100) and Nickel(111) Surfaces Molecular Orientation in Thin Monolayer Films by Infrared Spectroscopy Applications of Surface Polaritons for Detection and Vibrational SpectraSurface Raman Ellipsometry Fourier Transform Infrared Reflection-Absorption Spectroscopy of Surface Species The Adsorption of CO on Pt(111) Studied by Infrared-Reflection-Adsorption Spectroscopy Infrared-Spectroscopic Investigation of the Adsorption of Fluoromethane on Sodium Chloride Surfaces under Ultra High Vacuum Electroreflectance Vibrational Spectroscopy: A New Surface Analysis Technique Using Diode Lasers Infrared Spectra of CO Adsorbed at Low Temperatures on NiSession VII: Beam-Surface Scattering
  • Surface Phonons The Spectroscopy of Surface Vibrations by Atom Scattering Internal State Distributions of Molecules Scattering and Desorbing from Surfaces Hydrogen Interactions with Ag(111): Bound State Scattering Resonances and Interaction Potential Determination Ro-Vibrational Excitation within the Infinite Conical Well: Desorption of Diatomic Molecules X-Ray and Neutron Diffraction Measurements on Physisorbed Films on Graphite Surface Phonons in Superlattices Bound States of Two Surface Phonons at a Crystal Surface with an Adsorbed Monolayer A Search for High Frequency Vibrational Modes at a Stepped Surface Crystallographic Determination of Metal Surfaces with Helium Scattering Roughness-Trapped Shear Horizontal Surface Acoustic Waves Leaky Surface-Elastic Waves on Flat and Highly Corrugated Surfaces for Isotropic Non-dissipative Media Measurement of Au(111) Surface Phonons by Low Energy Helium ScatteringSession VIII: Electron Tunneling Spectroscopy
  • Surface Enhanced Raman Studies in Electrochemistry Tunneling Spectroscopy as a Probe of Adsorbate-Surface Interactions The Interaction of Ions and Easily Ionized Species with Oxide Surfaces as Studied by Tunneling Spectroscopy Surface Enhanced Raman Scattering of Water on an Ag Electrode EMIRS Study of Adsorbate Bonding in the Electrode Solution Interfacial Region Spectral Properties of Pyrazine Adsorbed on Silver Electrodes and Cold Silver Films from Surface Enhanced Raman Scattering (SERS) SERS Study of Pyridine Vapor Exposed to Silver Substrates Electrochemically Prepared Experimental Study of Relative Intensities in Inelastic Electron Tunneling Spectroscopy (I.E.T.S.) Study of Adsorption of the Electrode/Solution Interphase by In-Situ Infrared Reflectance Spectroscopy - Adsorption of Methanol on a Platinum Electrode Intensity Enhancement and Spectral Change in Raman Scattering of Mercaptobenzothiazole Adsorbed on Silver Electrode Time Dependence of Surface Enhanced Raman Scattering During and After Oxidation-Reduction CyclesSession IX: Conference Summary and Outlook Conference Overview, Directions for Future Work and Critical Issues: Theory Conference Overview: ExperimentalLiterature Reviews Infrared Investigations of Adsorbed Species on Films and Monocrystalline Surfaces: A literature search Vibrations Measured at Surfaces by HREELS: An updated review A Tabular Review of Tunneling Spectroscopy Raman Spectra of Molecules Considered to be Surface EnhancedAuthor IndexSubject Index

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