Electron transfer : from isolated molecules to biomolecules
著者
書誌事項
Electron transfer : from isolated molecules to biomolecules
（Advances in chemical physics / edited by I. Prigogine and Stuart A. Rice, v. 106-107）
Wiley, c1999
- part 1
- part 2
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注記
An Interscience publication
Includes bibliographical references and indexes
内容説明・目次
- 巻冊次
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part 2 ISBN 9780471252917
内容説明
an integrated approach to electron transfer phenomena
This two-part stand-alone volume in the prestigious Advances in Chemical Physics series provides the most comprehensive overview of electron transfer science today. It draws on cutting-edge research from diverse areas of chemistry, physics, and biology-covering the most recent developments in the field, and pointing to important future trends. This second volume offers the following sections:
* Solvent control, including ultrafast solvation dynamics and related topics
* Ultrafast electron transfer and coherence effects
* Molecular electronics
* Electron transfer and exciplex chemistry
* Biomolecules-from electron transfer tubes to kinetics in a DNA environment
Part One addresses the historical perspective, electron transfer phenomena in isolated molecules and clusters, general theory, and electron transfer kinetics in bridged compounds.
Electron transfer science has seen tremendous progress in recent years. Technological innovations, most notably the advent of femtosecond lasers, now permit the real-time investigation of intramolecular and intermolecular electron transfer processes on a time scale of nuclear motion. New scientific information abounds, illuminating the processes of energy acquisition, storage, and disposal in large molecules, clusters, condensed phase, and biophysical systems.
Electron Transfer: From Isolated Molecules to Biomolecules is the first book devoted to the exciting work being done in nonradiative electron transfer dynamics today. This two-part edited volume emphasizes the interdisciplinary nature of the field, bringing together the contributions of pioneers in chemistry, physics, and biology. Both theoretical and experimental topics are featured. The authors describe modern approaches to the exploration of different systems, including supersonic beam techniques, femtosecond laser spectroscopy, chemical syntheses, and methods in genetic and chemical engineering. They examine applications in such areas as supersonic jets, solvents, electrodes, semi- conductors, respiratory and enzymatic protein systems, photosynthesis, and more. They also relate electron transfer and radiationless transitions theory to pertinent physical phenomena, and provide a conceptual framework for the different processes.
Complete with over two hundred illustrations, Part Two opens with solvent control issues, including electron transfer reactions and ultrafast solvation dynamics. Other topics include ultrafast electron transfer and coherence effects, molecular electronics, and electron transfer in exciplex chemistry. This volume concludes with a section on biomolecules-from electron transfer tubes to experimental electron transfer and transport in DNA.
Timely, comprehensive, and authoritative, Electron Transfer: From Isolated Molecules to Biomolecules is an essential resource for physical chemists, molecular physicists, and researchers working in nonradiative dynamics today.
目次
Interplay Between Ultrafast Polar Solvation and Vibrational Dynamics in Electron Transfer Reactions: Role of High-Frequency Vibrational Modes (B. Bagchi & N. Gayathri).
Solvent Control of Electron Transfer Reactions (F. Raineri & H. Friedman).
Theoretical and Experimental Study of Ultrafast Solvation Dynamics by Transient Four-Photon Spectroscopy (B. Fainberg & D. Huppert).
Coherence and Adiabaticity in Ultrafast Electron Transfer (K. Wynne & R. Hochstrasser).
Electron Transfer and Solvent Dynamics in Two- and Three-State Systems (M. Cho & G. Fleming).
Ultrafast Intermolecular Electron Transfer in Solution (K. Yoshihara).
Electron Transfer in Molecules and Molecular Wires: Geometry Dependence, Coherent Transfer, and Control (V. Mujica, et al.).
Electron Transfer and Exciplex Chemistry (N. Mataga & H. Miyasaka).
Electron-Transfer Tubes (J. Regan & J. Onuchic).
Copper Proteins as Model Systems for Investigating Intramolecular Electron Transfer Processes (O. Farver & I. Pecht).
Applying Marcus's Theory to Electron Transfer in Vivo (G. McLendon, et al.).
Solvent-Fluctuation Control of Solution Reactions and Its Manifestation in Protein Functions (H. Sumi).
Experimental Electron Transfer Kinetics in a DNA Environment (P. Barbara & E. Olson).
Indexes.
- 巻冊次
-
part 1 ISBN 9780471252924
内容説明
an integrated approach to electron transfer phenomena
This two-part stand-alone volume in the prestigious Advances in Chemical Physics series provides the most comprehensive overview of electron transfer science today. It draws on cutting-edge research from diverse areas of chemistry, physics, and biology-covering the most recent developments in the field, and pointing to important future trends. This initial volume includes:
* A historical perspective spanning five decades
* A review of concepts, problems, and ideas in current research
* Electron transfer in isolated molecules and in clusters
* General theory, including useful algorithms
* Spectra and electron transfer kinetics in bridged compounds
The second volume covers solvent control, ultrafast electron transfer and coherence effects, molecular electronics, electron transfer and chemistry, and biomolecules.
Electron transfer science has seen tremendous progress in recent years. Technological innovations, most notably the advent of femtosecond lasers, now permit the real-time investigation of intramolecular and intermolecular electron transfer processes on a time scale of nuclear motion. New scientific information abounds, illuminating the processes of energy acquisition, storage, and disposal in large molecules, clusters, condensed phase, and biophysical systems.
Electron Transfer: From Isolated Molecules to Biomolecules is the first book devoted to the exciting work being done in nonradiative electron transfer dynamics today. This two-part edited volume emphasizes the interdisciplinary nature of the field, bringing together the contributions of pioneers in chemistry, physics, and biology. Both theoretical and experimental topics are featured. The authors describe modern approaches to the exploration of different systems, including supersonic beam techniques, femtosecond laser spectroscopy, chemical syntheses, and methods in genetic and chemical engineering. They examine applications in such areas as supersonic jets, solvents, electrodes, semi- conductors, respiratory and enzymatic protein systems, photosynthesis, and more. They also relate electron transfer and radiationless transitions theory to pertinent physical phenomena, and provide a conceptual framework for the different processes.
Complete with over two hundred illustrations, Part One reviews developments in the field since its inception fifty years ago, and discusses electron transfer phenomena in both isolated molecules and in clusters. It outlines the general theory, exploring areas of the control of kinetics, structure-function relationships, fluctuations, coherence, and coupling to solvents with complex spectral density in different types of electron transfer processes.
Timely, comprehensive, and authoritative, Electron Transfer: From Isolated Molecules to Biomolecules is an essential resource for physical chemists, molecular physicists, and researchers working in nonradiative dynamics today.
目次
Electron Transfer Past and Future (R. Marcus).
Electron Transfer Reactions in Solution: A Historical Perspective (N. Sutin).
Electron Transfer-From Isolated Molecules to Biomolecules (M. Bixon & J. Jortner).
Charge Transfer in Bichromophoric Molecules in the Gas Phase (D. Levy).
Long-Range Charge Separation in Solvent-Free Donor-Bridge-Acceptor Systems (B. Wegewijs & J. Verhoeven).
Electron Transfer and Charge Separation in Clusters (C. Dessent, et al.).
Control of Electron Transfer Kinetics: Models for Medium Reorganization and Donor-Acceptor Coupling (M. Newton).
Theories of Structure-Function Relationships for Bridge-Mediated Electron Transfer Reactions (S. Skourtis & D. Beratan).
Fluctuations and Coherence in Long-Range and Multicenter Electron Transfer (G. Iversen, et al.).
Lanczos Algorithm for Electron Transfer Rates in Solvents with Complex Spectral Densities (A. Okada, et al.).
Spectroscopic Determination of Electron Transfer Barriers and Rate Constants (K. Omberg, et al.).
Photoinduced Electron Transfer Within Donor-Spacer-Acceptor Molecular Assemblies Studied by Time-Resolved Microwave Conductivity (J. Warman, et al.).
From Close Contact to Long-Range Intramolecular Electron Transfer (J. Verhoeven).
Photoinduced Electron Transfers Through Bonds in Solution (N.-C. Yang, et al.).
Indexes.
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