Synthesis of Benzene from Methane and Carbon Monoxide over Silica-Supported Rh, Ru and Pd Catalysts

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  • Shuichi Naito
    Department of Applied Chemistry, Faculty of Engineering, Kanagawa University3-27-1, Rokkakubashi, Kanagawa-ku, Yokohama
  • Tadahiko Karaki
    Department of Applied Chemistry, Faculty of Engineering, Kanagawa University3-27-1, Rokkakubashi, Kanagawa-ku, Yokohama
  • Toshiaki Iritani
    Department of Applied Chemistry, Faculty of Engineering, Kanagawa University3-27-1, Rokkakubashi, Kanagawa-ku, Yokohama

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Abstract

<jats:title>Abstract</jats:title> <jats:p>Benzene was formed selectively among hydrocarbons produced in CH4-CO reaction over silica supported Rh, Ru and Pd catalysts at 573-723 K under atmospheric pressures, although CO2 was the main product, which was formed by the disproportionation of CO. Addition of H2 to CH4-CO reaction accelerated the rate of benzene formation several times, and the selectivity increased considerably.</jats:p>

Journal

  • Chemistry Letters

    Chemistry Letters 26 (9), 877-878, 1997-09-01

    Oxford University Press (OUP)

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